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Trumotion look like crap to me in any mode, and I always disable most processing since it always makes things worse. The only two good processing options are Real Motion and dynamic tone mapping. PC mode will only work right for SDR, it always uses REC 709 for HDR (unless you have the fix in the 2018 models). RGB 4:4:4 is important because that's what madVR and the video process in, anything else will require conversion. HDR mode will require taking this hit, but I let my TV process from 4:4:4 to 4:2:2.
I do leave pixel shifting and ASBL enabled since neither effect movies or games, I could see where this could be an issue if you use the TV as a monitor. I have a separate monitor for normal computer functions (everything but movies/games).
FYI, there should be no additional calibrations required going to PC mode, whatever ISF calibrations you set will be exactly the same in PC (although you might need to set them).
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